Swelling, states of water, morphology, stability in the aqueous solution, and electro-mechano-chemical bending behaviors of the gelatin–chitosan blend system were studied in order to clarify the potential use of this blend system as an actuator. The gelatin–chitosan blend system was prepared in order to avoid dissolution of the pure chitosan in an aqueous medium and the rigidity and easy degradation of the pure gelatin in the swollen state.